Solution-Processed Mixed-Dimensional Hybrid Perovskite/Carbon Nanotube Electronics.

Chun Ma, Sarah Clark, Zhixiong Liu, Liangliang Liang, Yuliar Firdaus, Ran Tao, Ali Han, Xiaogang Liu, Lain-Jong Li, Thomas D. Anthopoulos, Mark C Hersam, Tao Wu

Research output: Contribution to journalArticlepeer-review

10 Scopus citations

Abstract

Benefiting from their extraordinary physical properties, methylammonium lead halide perovskites (PVKs) have attracted significant attention in optoelectronics. However, the PVK-based devices suffer from low carrier mobility and high operation voltage. Here, we utilize sorted semiconducting single-walled carbon nanotubes (95% s-SWCNTs) to enhance the performance of thin-film transistors (TFTs) based on the mixed-cation perovskite (MA1-xFAx)Pb(I1-xBrx)3, enabling mixed-dimensional solution-processed electronics with high mobility (32.25 cm2/(V s)) and low voltage (∼3 V) operation. The resulting mixed-dimensional PVK/SWCNT TFTs possess ON/OFF ratios on the order of 107, enabling the fabrication of high-gain inverters.
Original languageEnglish (US)
Pages (from-to)3969-3979
Number of pages11
JournalACS nano
Volume14
Issue number4
DOIs
StatePublished - Mar 3 2020

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