Made-to-order porous electrodes for supercapacitors: MOFs embedded with redox-active centers as a case study.

Arijit Mallick, Hanfeng Liang, Osama Shekhah, Jiangtao Jia, Georges Mouchaham, Aleksander Shkurenko, Youssef Belmabkhout, Husam N. Alshareef, Mohamed Eddaoudi

Research output: Contribution to journalArticlepeer-review

9 Scopus citations

Abstract

In this work, a pre-designed Zr-based-MOF encompassing an organic linker with a redox active core is synthesized and its structure-property relationship as a supercapacitor electrode is investigated. An enhanced performance is revealed by the combination of this MOF's high porosity and redox core incorporation, which alters its double-layer and pseudocapacitance, respectively. An increase in the capacitance performance by a factor of two is achieved via post-synthetic structure rigidification using organic pillars.
Original languageEnglish (US)
Pages (from-to)1883-1886
Number of pages4
JournalChemical communications (Cambridge, England)
Volume56
Issue number12
DOIs
StatePublished - 2020

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