High-performance nanostructured supercapacitors on a sponge

Wei Chen, Rakhi Raghavan Baby, Liangbing Hu, Xing Xie, Yi Cui, Husam N. Alshareef

Research output: Contribution to journalArticlepeer-review

610 Scopus citations

Abstract

A simple and scalable method has been developed to fabricate nanostructured MnO 2-carbon nanotube (CNT)-sponge hybrid electrodes. A novel supercapacitor, henceforth referred to as "sponge supercapacitor", has been fabricated using these hybrid electrodes with remarkable performance. A specific capacitance of 1230 F/g (based on the mass of MnO 2) can be reached. Capacitors based on CNT-sponge substrates (without MnO 2) can be operated even under a high scan rate of 200 V/s, and they exhibit outstanding cycle performance with only 2% degradation after 100000 cycles under a scan rate of 10 V/s. The MnO 2-CNT-sponge supercapacitors show only 4% of degradation after 10000 cycles at a charge-discharge specific current of 5 A/g. The specific power and energy of the MnO 2-CNT-sponge supercapacitors are high with values of 63 kW/kg and 31 Wh/kg, respectively. The attractive performances exhibited by these sponge supercapacitors make them potentially promising candidates for future energy storage systems. © 2011 American Chemical Society.
Original languageEnglish (US)
Pages (from-to)5165-5172
Number of pages8
JournalNano Letters
Volume11
Issue number12
DOIs
StatePublished - Dec 14 2011

ASJC Scopus subject areas

  • Bioengineering
  • Materials Science(all)
  • Chemistry(all)
  • Mechanical Engineering
  • Condensed Matter Physics

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