Dynamical study of a polydisperse hard-sphere system

Tomoaki Nogawa, Nobuyasu Ito, Hiroshi Watanabe

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9 Scopus citations

Abstract

We study the interplay between the fluid-crystal transition and the glass transition of elastic sphere system with polydispersity using nonequilibrium molecular dynamics simulations. It is found that the end point of the crystal-fluid transition line, which corresponds to the critical polydispersity above which the crystal state is unstable, is on the glass transition line. This means that crystal and fluid states at the melting point becomes less distinguishable as polydispersity increases and finally they become identical state, i.e., marginal glass state, at critical polydispersity. © 2010 The American Physical Society.
Original languageEnglish (US)
JournalPhysical Review E
Volume82
Issue number2
DOIs
StatePublished - Aug 10 2010
Externally publishedYes

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