Correlation of Photoluminescence and Structural Morphologies at the Individual Nanoparticle Level

Luis Gutiérrez-Arzaluz, Ghada H. Ahmed, Haoze Yang, Semen Shikin, Osman Bakr, Anton V. Malko, Omar F. Mohammed

Research output: Contribution to journalArticlepeer-review

1 Scopus citations

Abstract

Single-particle spectroscopy have demonstrated great potential for analyzing the microscopic behavior of various nanoparticles (NPs). However, high-resolution optical imaging of these materials at the nanoscale is still very challenging. Here, we present an experimental setup that combines the high sensitivity of time-correlated single-photon counting (TCSPC) techniques with atomic force microscopy (AFM). This system enabled us to have a single-photon emitter detection with a time resolution of 120 ps and a spatial resolution of 5 nm. We utilized our setup to investigate the photoluminescence (PL) characteristics of both zero-dimensional (0D) and threedimensional (3D) perovskite nanocrystals (PNCs) and establish a correlation between the particle’s sizes, their PL blinking, and the lifetime behavior. Our system demonstrates an unprecedented level of information, opening the door to understanding the morphology-luminescence correlation of various nanosystems.
Original languageEnglish (US)
Pages (from-to)4855-4860
Number of pages6
JournalThe Journal of Physical Chemistry A
Volume124
Issue number23
DOIs
StatePublished - May 12 2020

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