Amplification of Surface-Enhanced Raman Scattering Due to Substrate-Mediated Localized Surface Plasmons in Gold Nanodimers

Weisheng Yue, Zhihong Wang, John Whittaker, Francisco Lopez-royo, Yang Yang, Anatoly Zayats

    Research output: Contribution to journalArticlepeer-review

    29 Scopus citations

    Abstract

    Surface-enhanced Raman scattering (SERS) is ubiquitous in chemical and biochemical sensing, imaging and identification. Maximizing SERS enhancement is a continuous effort focused on the design of appropriate SERS substrates. Here we show that significant improvement in a SERS signal can be achieved with substrates combining localized surface plasmon resonances and a nonresonant plasmonic substrate. By introducing a continuous gold (Au) film underneath Au nanodimers antenna arrays, an over 10-fold increase in SERS enhancement is demonstrated. Triangular, rectangle and disc dimers were studied, with bowtie antenna providing highest SERS enhancement. Simulations of electromagnetic field distributions of the Au nanodimers on the Au film support the observed enhancement dependences. The hybridization of localized plasmonic modes with the image modes in a metal film provides a straightforward way to improve SERS enhancement in designer SERS substrate.
    Original languageEnglish (US)
    Pages (from-to)4075-4084
    Number of pages10
    JournalJ. Mater. Chem. C
    Volume5
    Issue number16
    DOIs
    StatePublished - 2017

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